我院王欣鹏副教授团队在共价有机框架材料高选择性分离锕系金属离子方面取得进展-特色金属材料与组合结构全寿命安全国家重点实验室

我院王欣鹏副教授团队在共价有机框架材料高选择性分离锕系金属离子方面取得进展

2023年03月27日 15:53 资环材点击：[]

近日，我院王欣鹏副教授团队与高能所石伟群研究员合作在国际 TOP 期刊《 Chemical Engineering Journal 》（中科院一区， IF=16.744 ）发表了题为《 Tailored covalent organic framework with phosphorylation for boosting typical actinide adsorption under acidic conditions 》的研究论文。

共价有机框架材料（Covalent Organic Frameworks，COFs）是由C、H、O、N、B等轻元素组成的有机小分子通过动态可逆的共价化学键连接的晶态多孔材料。与非晶态的多孔材料相比具有高比表面积、良好的化学稳定性和高度有序的周期性结构等诸多优点，在气体储存与吸附、催化和环境污染物的去除方面具有高潜力和广泛的功能化应用前景。

本团队设计合成了具有六边形孔道的COF骨架TzDa，通过后合成修饰的方法得到磷酸功能化的TzDa-Phos，用于水溶液中的锕系金属离子的高选择性去除，并通过FT-IR、XPS和EXAFS详细解释了随酸度变化相互作用机理的变化。在近中性条件下，主要是P-O^-参与U(VI)的配位；随着酸度的升高，P-O^-完全质子化，在高酸度下，TzDa-Phos对U(VI)和Pu(IV)的吸附能力主要是由于磷酸功能化基团中的P=O。这项工作证明了COF材料在处理放射性废水方面的应用潜力，并有助于通过具有确定拓扑结构和化学成分的COF基材料来了解影响固相萃取行为的关键因素。

论文链接：https://doi.org/10.1016/j.cej.2023.142408

上一条：我院朱金良副教授在磷化锰增强锂硫电池正极研究方面取得进展下一条：我院冯庆革教授团队在农村生态环境中的污染物迁移转化机制研究方面取得重要进展

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'tid' => '1', 'pid' => '11', 'mid' => 'news', 'pids' => '0,11', 'name' => '科研队伍', 'dirname' => 'keyanduiwu', 'pdirname' => 'shouye/', 'child' => 1, 'disabled' => '0', 'ismain' => 1, 'childids' => '24,51,52,53,54', 'thumb' => '', 'show' => '1', 'content' => '', 'setting' => array ( 'disabled' => '0', 'linkurl' => '', 'getchild' => '0', 'notedit' => '0', 'urlrule' => 0, 'seo' => array ( 'list_title' => '[第{page}页{join}]{catpname}{join}{SITE_NAME}', 'list_keywords' => '', 'list_description' => '', ), 'template' => array ( 'pagesize' => '20', 'mpagesize' => '20', 'page' => 'page.html', 'list' => 'listimg.html', 'category' => 'listimg.html', 'search' => 'search.html', 'show' => 'show.html', ), 'cat_field' => NULL, 'module_field' => NULL, 'html' => 0, ), 'displayorder' => '0', 'pcatpost' => 0, 'topid' => '11', 'catids' => array ( 0 => '24', 1 => '51', 2 => '52', 3 => '53', 4 => '54', ), 'is_post' => 0, 'url' => 'http://wei.vialancer.com/index.php?c=category&id=24', 'total' => '请使用count标签查询', 'field' => array ( ), ), 25 => array ( 'id' => '25', 'tid' => '1', 'pid' => '11', 'mid' => 'news', 'pids' => '0,11', 'name' => '研究团队', 'dirname' => 'yjtd', 'pdirname' => 'shouye/', 'child' => 0, 'disabled' => '0', 'ismain' => 1, 'childids' => 25, 'thumb' => '', 'show' => '1', 'content' => '', 'setting' => array ( 'disabled' => '0', 'linkurl' => '', 'getchild' => '0', 'notedit' => '0', 'urlrule' => 0, 'seo' => array ( 'list_title' => '[第{page}页{join}]{catpname}{join}{SITE_NAME}', 'list_keywords' => '', 'list_description' => '', ), 'template' => array ( 'pagesize' => '20', 'mpagesize' => '20', 'page' => 'page.html', 'list' => 'list.html', 'category' => 'category.html', 'search' => 'search.html', 'show' => 'show.html', ), 'cat_field' => NULL, 'module_field' => NULL, 'html' => 0, ), 'displayorder' => '0', 'pcatpost' => 0, 'topid' => '11', 'catids' => array ( 0 => '25', ), 'is_post' => 1, 'url' => 'http://wei.vialancer.com/index.php?c=category&id=25', 'total' => '请使用count标签查询', 'field' => array ( ), ), )
urlrule	'/index.php?c=show&id=27&page=[page]'
fix_html_now_url	''
my_web_url	'http://wei.vialancer.com/index.php?c=show&id=27'
get	array ( 'c' => 'show', 'id' => '27', )

我院王欣鹏副教授团队在共价有机框架材料高选择性分离锕系金属离子方面取得进展

友情链接

联系我们

联系我们

Database (5 Queries across 0 Connection)

Views

运行时间：0.01ms

模板文件

引用提示

模板变量

Files ( 148 )

Routes

Events

History

View Data

Session User Data

Request ( HTTP/1.1 )

$_GET

Headers

Cookies

Response ( 200 - OK )

Headers

System Configuration

App.php	APPPATH/Config/App.php
Auto.php	FCPATH/App/Module/Config/Auto.php
Autoload.php	APPPATH/Config/Autoload.php
AutoloadConfig.php	APPPATH/System/Config/AutoloadConfig.php
Autoloader.php	APPPATH/System/Autoloader/Autoloader.php
BaseBuilder.php	APPPATH/System/Database/BaseBuilder.php
BaseCollector.php	APPPATH/System/Debug/Toolbar/Collectors/BaseCollector.php
BaseConfig.php	APPPATH/System/Config/BaseConfig.php
BaseConnection.php	APPPATH/System/Database/BaseConnection.php
BaseHandler.php	APPPATH/System/Cache/Handlers/BaseHandler.php
BaseResult.php	APPPATH/System/Database/BaseResult.php
BaseService.php	APPPATH/System/Config/BaseService.php
Builder.php	APPPATH/System/Database/MySQLi/Builder.php
Cache.php	APPPATH/Config/Cache.php
Cache.php	APPPATH/Extend/Cache.php
Cache.php	FCPATH/Fcms/Library/Cache.php
CacheFactory.php	APPPATH/System/Cache/CacheFactory.php
CacheInterface.php	APPPATH/System/Cache/CacheInterface.php
Category.php	FCPATH/App/Module/Action/Category.php
CliRenderer.php	APPPATH/System/ThirdParty/Kint/Renderer/CliRenderer.php
CodeIgniter.php	APPPATH/Extend/CodeIgniter.php
CodeIgniter.php	APPPATH/System/CodeIgniter.php
Common.php	APPPATH/System/Common.php
Config.php	APPPATH/System/Config/Config.php
Config.php	APPPATH/System/Database/Config.php
Connection.php	APPPATH/System/Database/MySQLi/Connection.php
ConnectionInterface.php	APPPATH/System/Database/ConnectionInterface.php
Constants.php	APPPATH/Config/Constants.php
Content.php	FCPATH/App/Module/Models/Content.php
Content.php	FCPATH/Fcms/Model/Content.php
ContentSecurityPolicy.php	APPPATH/Config/ContentSecurityPolicy.php
ContentSecurityPolicy.php	APPPATH/System/HTTP/ContentSecurityPolicy.php
Controller.php	APPPATH/Extend/Controller.php
Controller.php	APPPATH/System/Controller.php
Database.php	APPPATH/Config/Database.php
Database.php	APPPATH/System/Database/Database.php
Database.php	APPPATH/System/Debug/Toolbar/Collectors/Database.php
Date.php	FCPATH/Fcms/Field/Date.php
DebugToolbar.php	APPPATH/System/Filters/DebugToolbar.php
DotEnv.php	APPPATH/System/Config/DotEnv.php
Editor.php	FCPATH/Fcms/Field/Editor.php
Events.php	APPPATH/Config/Events.php
Events.php	APPPATH/System/Debug/Toolbar/Collectors/Events.php
Events.php	APPPATH/System/Events/Events.php
Exceptions.php	APPPATH/Config/Exceptions.php
Exceptions.php	APPPATH/Extend/Exceptions.php
Exceptions.php	APPPATH/System/Debug/Exceptions.php
Factories.php	APPPATH/System/Config/Factories.php
Factory.php	APPPATH/System/Config/Factory.php
Field.php	FCPATH/Fcms/Library/Field.php
File.php	FCPATH/Fcms/Field/File.php
FileHandler.php	APPPATH/System/Cache/Handlers/FileHandler.php
FileLocator.php	APPPATH/System/Autoloader/FileLocator.php
Files.php	APPPATH/System/Debug/Toolbar/Collectors/Files.php
FilterInterface.php	APPPATH/System/Filters/FilterInterface.php
Filters.php	APPPATH/Config/Filters.php
Filters.php	APPPATH/System/Filters/Filters.php
Header.php	APPPATH/System/HTTP/Header.php
Helper.php	FCPATH/Fcms/Core/Helper.php
Hook.php	APPPATH/Extend/Hook.php
Hooks.php	FCPATH/App/Module/Config/Hooks.php
Hooks.php	FCPATH/Fcms/Core/Hooks.php
IncomingRequest.php	APPPATH/System/HTTP/IncomingRequest.php
Init.php	APPPATH/Init.php
Init.php	FCPATH/Fcms/Init.php
Input.php	FCPATH/Fcms/Library/Input.php
Kint.php	APPPATH/Config/Kint.php
Kint.php	APPPATH/System/ThirdParty/Kint/Kint.php
Lang.php	FCPATH/Fcms/Library/Lang.php
Logger.php	APPPATH/Config/Logger.php
Logger.php	APPPATH/System/Log/Logger.php
LoggerInterface.php	APPPATH/System/ThirdParty/PSR/Log/LoggerInterface.php
Logs.php	APPPATH/System/Debug/Toolbar/Collectors/Logs.php
Member.php	FCPATH/Fcms/Model/Member.php
Message.php	APPPATH/System/HTTP/Message.php
MessageInterface.php	APPPATH/System/HTTP/MessageInterface.php
MessageTrait.php	APPPATH/System/HTTP/MessageTrait.php
Model.php	APPPATH/Extend/Model.php
Model.php	FCPATH/Fcms/Core/Model.php
Module.php	FCPATH/App/Module/Extends/Home/Module.php
Modules.php	APPPATH/Config/Modules.php
Modules.php	APPPATH/System/Modules/Modules.php
Paths.php	APPPATH/Config/Paths.php
Phpcmf.php	FCPATH/Fcms/Core/Phpcmf.php
Query.php	APPPATH/System/Database/Query.php
QueryInterface.php	APPPATH/System/Database/QueryInterface.php
Related.php	FCPATH/App/Module/Action/Related.php
Renderer.php	APPPATH/System/ThirdParty/Kint/Renderer/Renderer.php
RendererInterface.php	APPPATH/System/View/RendererInterface.php
Request.php	APPPATH/Extend/Request.php
Request.php	APPPATH/System/HTTP/Request.php
RequestInterface.php	APPPATH/System/HTTP/RequestInterface.php
RequestTrait.php	APPPATH/System/HTTP/RequestTrait.php
Response.php	APPPATH/System/HTTP/Response.php
ResponseInterface.php	APPPATH/System/HTTP/ResponseInterface.php
ResponseTrait.php	APPPATH/System/API/ResponseTrait.php
ResponseTrait.php	APPPATH/System/HTTP/ResponseTrait.php
Result.php	APPPATH/System/Database/MySQLi/Result.php
ResultInterface.php	APPPATH/System/Database/ResultInterface.php
RichRenderer.php	APPPATH/System/ThirdParty/Kint/Renderer/RichRenderer.php
RouteCollection.php	APPPATH/System/Router/RouteCollection.php
RouteCollectionInterface.php	APPPATH/System/Router/RouteCollectionInterface.php
Router.php	APPPATH/System/Router/Router.php
Router.php	FCPATH/Fcms/Library/Router.php
RouterInterface.php	APPPATH/System/Router/RouterInterface.php
Routes.php	APPPATH/Config/Routes.php
Routes.php	APPPATH/Extend/Routes.php
Routes.php	APPPATH/System/Config/Routes.php
Routes.php	APPPATH/System/Debug/Toolbar/Collectors/Routes.php
Security.php	FCPATH/Fcms/Library/Security.php
Seo.php	FCPATH/Fcms/Library/Seo.php
Service.php	FCPATH/Fcms/Core/Service.php
Services.php	APPPATH/Config/Services.php
Services.php	APPPATH/System/Config/Services.php
Show.php	FCPATH/Fcms/Control/Show.php
Text.php	FCPATH/Fcms/Field/Text.php
TextRenderer.php	APPPATH/System/ThirdParty/Kint/Renderer/TextRenderer.php
Textarea.php	FCPATH/Fcms/Field/Textarea.php
Timer.php	APPPATH/System/Debug/Timer.php
Timers.php	APPPATH/System/Debug/Toolbar/Collectors/Timers.php
Toolbar.php	APPPATH/Config/Toolbar.php
Toolbar.php	APPPATH/System/Debug/Toolbar.php
URI.php	APPPATH/System/HTTP/URI.php
UserAgent.php	APPPATH/System/HTTP/UserAgent.php
UserAgents.php	APPPATH/Config/UserAgents.php
Utils.php	APPPATH/System/ThirdParty/Kint/Utils.php
Version.php	FCPATH/My/Config/Version.php
View.php	APPPATH/Config/View.php
View.php	APPPATH/Extend/View.php
View.php	APPPATH/System/Config/View.php
View.php	APPPATH/System/View/View.php
View.php	FCPATH/Fcms/Core/View.php
Views.php	APPPATH/System/Debug/Toolbar/Collectors/Views.php
custom.php	/webdata/wei/config/custom.php
database.php	/webdata/wei/config/database.php
domain_app.php	/webdata/wei/cache/config/domain_app.php
domain_client.php	/webdata/wei/cache/config/domain_client.php
hooks.php	/webdata/wei/config/hooks.php
index.php	/webdata/wei/index.php
init.php	APPPATH/System/ThirdParty/Kint/init.php
init_helpers.php	APPPATH/System/ThirdParty/Kint/init_helpers.php
lang.php	/webdata/wei/api/language/zh-cn/lang.php
site.php	/webdata/wei/cache/config/site.php
system.php	/webdata/wei/cache/config/system.php
template_DS_pc_DS_default_DS_home_DS_footer.html.cache.php	/webdata/wei/cache/template/template_DS_pc_DS_default_DS_home_DS_footer.html.cache.php
template_DS_pc_DS_default_DS_home_DS_header.html.cache.php	/webdata/wei/cache/template/template_DS_pc_DS_default_DS_home_DS_header.html.cache.php
template_DS_pc_DS_default_DS_home_DS_show.html.cache.php	/webdata/wei/cache/template/template_DS_pc_DS_default_DS_home_DS_show.html.cache.php
url_helper.php	APPPATH/System/Helpers/url_helper.php

File:	/webdata/wei/dayrui/Fcms/Control/Show.php
App:	/
Controller:	show
Method:	index
URI:	show/index
URL:	http://wei.vialancer.com/index.php?c=show&id=27

Datetime	Status	Method	URL	Content-Type	Is AJAX?
2023-07-25 14:40:22	200	GET	http://wei.vialancer.com/	text/html; charset=UTF-8	No
2023-07-25 14:40:18	200	GET	http://wei.vialancer.com/	text/html; charset=UTF-8	No
2023-07-25 11:50:35	200	GET	http://wei.vialancer.com/	text/html; charset=UTF-8	No
2023-07-25 11:50:33	200	GET	http://wei.vialancer.com/	text/html; charset=UTF-8	No
2023-07-25 11:50:31	200	GET	http://wei.vialancer.com/	text/html; charset=UTF-8	No
2023-07-25 11:50:29	200	GET	http://wei.vialancer.com/	text/html; charset=UTF-8	No
2023-07-25 11:50:25	200	GET	http://wei.vialancer.com/	text/html; charset=UTF-8	No
2023-07-25 11:50:20	200	GET	http://wei.vialancer.com/	text/html; charset=UTF-8	No
2023-07-25 11:50:18	200	GET	http://wei.vialancer.com/	text/html; charset=UTF-8	No
2023-07-25 11:50:16	200	GET	http://wei.vialancer.com/	text/html; charset=UTF-8	No
2023-07-25 11:50:12	200	GET	http://wei.vialancer.com/	text/html; charset=UTF-8	No
2023-07-25 11:50:06	200	GET	http://wei.vialancer.com/	text/html; charset=UTF-8	No
2023-07-25 11:50:03	200	GET	http://wei.vialancer.com/	text/html; charset=UTF-8	No
2023-07-25 11:49:39	200	GET	http://wei.vialancer.com/	text/html; charset=UTF-8	No
2023-07-25 11:49:36	200	GET	http://wei.vialancer.com/	text/html; charset=UTF-8	No
2023-07-25 09:50:02	200	GET	http://wei.vialancer.com/	text/html; charset=UTF-8	No
2023-07-25 09:36:57	200	GET	http://wei.vialancer.com/	text/html; charset=UTF-8	No
2023-07-25 09:35:42	200	GET	http://wei.vialancer.com/	text/html; charset=UTF-8	No
2023-07-25 09:33:16	200	GET	http://wei.vialancer.com/	text/html; charset=UTF-8	No
2023-07-24 17:45:43	200	GET	http://wei.vialancer.com/	text/html; charset=UTF-8	No

Cookie	pgv_pvi=2798497912
Accept-Language	zh-CN,zh;q=0.9
Accept-Encoding	gzip, deflate
Referer	http://wei.vialancer.com/index.php?c=category&id=12
Accept	text/html,application/xhtml+xml,application/xml;q=0.9,image/avif,image/webp,image/apng,/;q=0.8,application/signed-exchange;v=b3;q=0.7
User-Agent	Mozilla/5.0 (Windows NT 10.0; Win64; x64) AppleWebKit/537.36 (KHTML, like Gecko) Chrome/113.0.0.0 Safari/537.36
Upgrade-Insecure-Requests	1
Connection	keep-alive
Host	wei.vialancer.com

CodeIgniter Version:	4.0.5
PHP Version:	7.2.16
PHP SAPI:	fpm-fcgi
Environment:	development
Base URL:	http://wei.vialancer.com/
Timezone:	PRC
Locale:	en
Content Security Policy Enabled:	No

Time	Event Name	Times Called
4.91 ms	pre_system	1
0.05 ms	dbquery	5

我院王欣鹏副教授团队在共价有机框架材料高选择性分离锕系金属离子方面取得进展

友情链接

联系我们

联系我们

4.0.5

Database (5 Queries across 0 Connection)

Views

运行时间：0.01ms

模板文件

引用提示

模板变量

Files ( 148 )

Routes

Events

History

View Data

Session User Data

Request ( HTTP/1.1 )

$_GET

Headers

Cookies

Response ( 200 - OK )

Headers

System Configuration