省部共建国重室刘熙俊教授团队在通过偶联还原二氧化碳和硝酸盐高效尿素生产的FeCu双金属簇方面取得进展-特色金属材料与组合结构全寿命安全国家重点实验室

省部共建国重室刘熙俊教授团队在通过偶联还原二氧化碳和硝酸盐高效尿素生产的FeCu双金属簇方面取得进展

2024年07月04日 09:53 点击：[]

近日，省部共建国重室刘熙俊教授团队在通过偶联还原二氧化碳和硝酸盐高效尿素生产的FeCu双金属簇方面取得进展，相关工作以"FeCu bimetallic clusters for efficient urea production via coupling reduction of carbon dioxide and nitrate"为题，发表在《Journal of Colloid and Interface Science》上。

尿素电合成具有满足氮循环和碳中和、节能的特点。铜可以与CO₂和氮气共电催化生成尿素，但开发有效的电催化剂仍是一个障碍。在此，我们开发了一种负载FeCu簇的氮掺杂多孔碳，将CO₂和NO3^-转化为尿素，其法拉第效率最高为39.8%，产率为1024.6 μg h⁻¹mgcat⁻¹。在优化的环境条件下，大于Fe或Cu均相位点。此外，通过原位傅里叶变换红外光谱和理论计算，还验证了在铁铜双活性位点上，*NHCO 和 *NHCONO 这两个中间产物具有较低的自由能垒，从而形成了有利的 Csingle bondN 偶联途径。这项研究可为深入了解耦合机理和研究绿色尿素生产的高效催化剂提供帮助。

上一条：省部共建国重室王欣鹏团队在改善光催化制氢和降解亚甲基蓝方面取得进展下一条：省部共建国重室王欣鹏团队在脱除水中盐酸四环素方面取得进展

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'field' => array ( ), ), 25 => array ( 'id' => '25', 'tid' => '1', 'pid' => '11', 'mid' => 'news', 'pids' => '0,11', 'name' => '研究团队', 'dirname' => 'yjtd', 'pdirname' => 'shouye/', 'child' => 0, 'disabled' => '0', 'ismain' => 1, 'childids' => 25, 'thumb' => '', 'show' => '1', 'content' => '', 'setting' => array ( 'disabled' => '0', 'linkurl' => '', 'getchild' => '0', 'notedit' => '0', 'urlrule' => 0, 'seo' => array ( 'list_title' => '[第{page}页{join}]{catpname}{join}{SITE_NAME}', 'list_keywords' => '', 'list_description' => '', ), 'template' => array ( 'pagesize' => '20', 'mpagesize' => '20', 'page' => 'page.html', 'list' => 'list.html', 'category' => 'category.html', 'search' => 'search.html', 'show' => 'show.html', ), 'cat_field' => NULL, 'module_field' => NULL, 'html' => 0, ), 'displayorder' => '0', 'pcatpost' => 0, 'topid' => '11', 'catids' => array ( 0 => '25', ), 'is_post' => 1, 'url' => 'http://wei.vialancer.com/index.php?c=category&id=25', 'total' => '请使用count标签查询', 'field' => array ( ), ), )
urlrule	'/index.php?c=show&id=27&page=[page]'
fix_html_now_url	''
my_web_url	'http://wei.vialancer.com/index.php?c=show&id=27'
get	array ( 'c' => 'show', 'id' => '27', )

Files ( 148 )

App.php	APPPATH/Config/App.php
Auto.php	FCPATH/App/Module/Config/Auto.php
Autoload.php	APPPATH/Config/Autoload.php
AutoloadConfig.php	APPPATH/System/Config/AutoloadConfig.php
Autoloader.php	APPPATH/System/Autoloader/Autoloader.php
BaseBuilder.php	APPPATH/System/Database/BaseBuilder.php
BaseCollector.php	APPPATH/System/Debug/Toolbar/Collectors/BaseCollector.php
BaseConfig.php	APPPATH/System/Config/BaseConfig.php
BaseConnection.php	APPPATH/System/Database/BaseConnection.php
BaseHandler.php	APPPATH/System/Cache/Handlers/BaseHandler.php
BaseResult.php	APPPATH/System/Database/BaseResult.php
BaseService.php	APPPATH/System/Config/BaseService.php
Builder.php	APPPATH/System/Database/MySQLi/Builder.php
Cache.php	APPPATH/Config/Cache.php
Cache.php	APPPATH/Extend/Cache.php
Cache.php	FCPATH/Fcms/Library/Cache.php
CacheFactory.php	APPPATH/System/Cache/CacheFactory.php
CacheInterface.php	APPPATH/System/Cache/CacheInterface.php
Category.php	FCPATH/App/Module/Action/Category.php
CliRenderer.php	APPPATH/System/ThirdParty/Kint/Renderer/CliRenderer.php
CodeIgniter.php	APPPATH/Extend/CodeIgniter.php
CodeIgniter.php	APPPATH/System/CodeIgniter.php
Common.php	APPPATH/System/Common.php
Config.php	APPPATH/System/Config/Config.php
Config.php	APPPATH/System/Database/Config.php
Connection.php	APPPATH/System/Database/MySQLi/Connection.php
ConnectionInterface.php	APPPATH/System/Database/ConnectionInterface.php
Constants.php	APPPATH/Config/Constants.php
Content.php	FCPATH/App/Module/Models/Content.php
Content.php	FCPATH/Fcms/Model/Content.php
ContentSecurityPolicy.php	APPPATH/Config/ContentSecurityPolicy.php
ContentSecurityPolicy.php	APPPATH/System/HTTP/ContentSecurityPolicy.php
Controller.php	APPPATH/Extend/Controller.php
Controller.php	APPPATH/System/Controller.php
Database.php	APPPATH/Config/Database.php
Database.php	APPPATH/System/Database/Database.php
Database.php	APPPATH/System/Debug/Toolbar/Collectors/Database.php
Date.php	FCPATH/Fcms/Field/Date.php
DebugToolbar.php	APPPATH/System/Filters/DebugToolbar.php
DotEnv.php	APPPATH/System/Config/DotEnv.php
Editor.php	FCPATH/Fcms/Field/Editor.php
Events.php	APPPATH/Config/Events.php
Events.php	APPPATH/System/Debug/Toolbar/Collectors/Events.php
Events.php	APPPATH/System/Events/Events.php
Exceptions.php	APPPATH/Config/Exceptions.php
Exceptions.php	APPPATH/Extend/Exceptions.php
Exceptions.php	APPPATH/System/Debug/Exceptions.php
Factories.php	APPPATH/System/Config/Factories.php
Factory.php	APPPATH/System/Config/Factory.php
Field.php	FCPATH/Fcms/Library/Field.php
File.php	FCPATH/Fcms/Field/File.php
FileHandler.php	APPPATH/System/Cache/Handlers/FileHandler.php
FileLocator.php	APPPATH/System/Autoloader/FileLocator.php
Files.php	APPPATH/System/Debug/Toolbar/Collectors/Files.php
FilterInterface.php	APPPATH/System/Filters/FilterInterface.php
Filters.php	APPPATH/Config/Filters.php
Filters.php	APPPATH/System/Filters/Filters.php
Header.php	APPPATH/System/HTTP/Header.php
Helper.php	FCPATH/Fcms/Core/Helper.php
Hook.php	APPPATH/Extend/Hook.php
Hooks.php	FCPATH/App/Module/Config/Hooks.php
Hooks.php	FCPATH/Fcms/Core/Hooks.php
IncomingRequest.php	APPPATH/System/HTTP/IncomingRequest.php
Init.php	APPPATH/Init.php
Init.php	FCPATH/Fcms/Init.php
Input.php	FCPATH/Fcms/Library/Input.php
Kint.php	APPPATH/Config/Kint.php
Kint.php	APPPATH/System/ThirdParty/Kint/Kint.php
Lang.php	FCPATH/Fcms/Library/Lang.php
Logger.php	APPPATH/Config/Logger.php
Logger.php	APPPATH/System/Log/Logger.php
LoggerInterface.php	APPPATH/System/ThirdParty/PSR/Log/LoggerInterface.php
Logs.php	APPPATH/System/Debug/Toolbar/Collectors/Logs.php
Member.php	FCPATH/Fcms/Model/Member.php
Message.php	APPPATH/System/HTTP/Message.php
MessageInterface.php	APPPATH/System/HTTP/MessageInterface.php
MessageTrait.php	APPPATH/System/HTTP/MessageTrait.php
Model.php	APPPATH/Extend/Model.php
Model.php	FCPATH/Fcms/Core/Model.php
Module.php	FCPATH/App/Module/Extends/Home/Module.php
Modules.php	APPPATH/Config/Modules.php
Modules.php	APPPATH/System/Modules/Modules.php
Paths.php	APPPATH/Config/Paths.php
Phpcmf.php	FCPATH/Fcms/Core/Phpcmf.php
Query.php	APPPATH/System/Database/Query.php
QueryInterface.php	APPPATH/System/Database/QueryInterface.php
Related.php	FCPATH/App/Module/Action/Related.php
Renderer.php	APPPATH/System/ThirdParty/Kint/Renderer/Renderer.php
RendererInterface.php	APPPATH/System/View/RendererInterface.php
Request.php	APPPATH/Extend/Request.php
Request.php	APPPATH/System/HTTP/Request.php
RequestInterface.php	APPPATH/System/HTTP/RequestInterface.php
RequestTrait.php	APPPATH/System/HTTP/RequestTrait.php
Response.php	APPPATH/System/HTTP/Response.php
ResponseInterface.php	APPPATH/System/HTTP/ResponseInterface.php
ResponseTrait.php	APPPATH/System/API/ResponseTrait.php
ResponseTrait.php	APPPATH/System/HTTP/ResponseTrait.php
Result.php	APPPATH/System/Database/MySQLi/Result.php
ResultInterface.php	APPPATH/System/Database/ResultInterface.php
RichRenderer.php	APPPATH/System/ThirdParty/Kint/Renderer/RichRenderer.php
RouteCollection.php	APPPATH/System/Router/RouteCollection.php
RouteCollectionInterface.php	APPPATH/System/Router/RouteCollectionInterface.php
Router.php	APPPATH/System/Router/Router.php
Router.php	FCPATH/Fcms/Library/Router.php
RouterInterface.php	APPPATH/System/Router/RouterInterface.php
Routes.php	APPPATH/Config/Routes.php
Routes.php	APPPATH/Extend/Routes.php
Routes.php	APPPATH/System/Config/Routes.php
Routes.php	APPPATH/System/Debug/Toolbar/Collectors/Routes.php
Security.php	FCPATH/Fcms/Library/Security.php
Seo.php	FCPATH/Fcms/Library/Seo.php
Service.php	FCPATH/Fcms/Core/Service.php
Services.php	APPPATH/Config/Services.php
Services.php	APPPATH/System/Config/Services.php
Show.php	FCPATH/Fcms/Control/Show.php
Text.php	FCPATH/Fcms/Field/Text.php
TextRenderer.php	APPPATH/System/ThirdParty/Kint/Renderer/TextRenderer.php
Textarea.php	FCPATH/Fcms/Field/Textarea.php
Timer.php	APPPATH/System/Debug/Timer.php
Timers.php	APPPATH/System/Debug/Toolbar/Collectors/Timers.php
Toolbar.php	APPPATH/Config/Toolbar.php
Toolbar.php	APPPATH/System/Debug/Toolbar.php
URI.php	APPPATH/System/HTTP/URI.php
UserAgent.php	APPPATH/System/HTTP/UserAgent.php
UserAgents.php	APPPATH/Config/UserAgents.php
Utils.php	APPPATH/System/ThirdParty/Kint/Utils.php
Version.php	FCPATH/My/Config/Version.php
View.php	APPPATH/Config/View.php
View.php	APPPATH/Extend/View.php
View.php	APPPATH/System/Config/View.php
View.php	APPPATH/System/View/View.php
View.php	FCPATH/Fcms/Core/View.php
Views.php	APPPATH/System/Debug/Toolbar/Collectors/Views.php
custom.php	/webdata/wei/config/custom.php
database.php	/webdata/wei/config/database.php
domain_app.php	/webdata/wei/cache/config/domain_app.php
domain_client.php	/webdata/wei/cache/config/domain_client.php
hooks.php	/webdata/wei/config/hooks.php
index.php	/webdata/wei/index.php
init.php	APPPATH/System/ThirdParty/Kint/init.php
init_helpers.php	APPPATH/System/ThirdParty/Kint/init_helpers.php
lang.php	/webdata/wei/api/language/zh-cn/lang.php
site.php	/webdata/wei/cache/config/site.php
system.php	/webdata/wei/cache/config/system.php
template_DS_pc_DS_default_DS_home_DS_footer.html.cache.php	/webdata/wei/cache/template/template_DS_pc_DS_default_DS_home_DS_footer.html.cache.php
template_DS_pc_DS_default_DS_home_DS_header.html.cache.php	/webdata/wei/cache/template/template_DS_pc_DS_default_DS_home_DS_header.html.cache.php
template_DS_pc_DS_default_DS_home_DS_show.html.cache.php	/webdata/wei/cache/template/template_DS_pc_DS_default_DS_home_DS_show.html.cache.php
url_helper.php	APPPATH/System/Helpers/url_helper.php

Routes

File:	/webdata/wei/dayrui/Fcms/Control/Show.php
App:	/
Controller:	show
Method:	index
URI:	show/index
URL:	http://wei.vialancer.com/index.php?c=show&id=27

Events

Time	Event Name	Times Called
4.91 ms	pre_system	1
0.05 ms	dbquery	5

History

Datetime	Status	Method	URL	Content-Type	Is AJAX?
2023-07-25 14:40:22	200	GET	http://wei.vialancer.com/	text/html; charset=UTF-8	No
2023-07-25 14:40:18	200	GET	http://wei.vialancer.com/	text/html; charset=UTF-8	No
2023-07-25 11:50:35	200	GET	http://wei.vialancer.com/	text/html; charset=UTF-8	No
2023-07-25 11:50:33	200	GET	http://wei.vialancer.com/	text/html; charset=UTF-8	No
2023-07-25 11:50:31	200	GET	http://wei.vialancer.com/	text/html; charset=UTF-8	No
2023-07-25 11:50:29	200	GET	http://wei.vialancer.com/	text/html; charset=UTF-8	No
2023-07-25 11:50:25	200	GET	http://wei.vialancer.com/	text/html; charset=UTF-8	No
2023-07-25 11:50:20	200	GET	http://wei.vialancer.com/	text/html; charset=UTF-8	No
2023-07-25 11:50:18	200	GET	http://wei.vialancer.com/	text/html; charset=UTF-8	No
2023-07-25 11:50:16	200	GET	http://wei.vialancer.com/	text/html; charset=UTF-8	No
2023-07-25 11:50:12	200	GET	http://wei.vialancer.com/	text/html; charset=UTF-8	No
2023-07-25 11:50:06	200	GET	http://wei.vialancer.com/	text/html; charset=UTF-8	No
2023-07-25 11:50:03	200	GET	http://wei.vialancer.com/	text/html; charset=UTF-8	No
2023-07-25 11:49:39	200	GET	http://wei.vialancer.com/	text/html; charset=UTF-8	No
2023-07-25 11:49:36	200	GET	http://wei.vialancer.com/	text/html; charset=UTF-8	No
2023-07-25 09:50:02	200	GET	http://wei.vialancer.com/	text/html; charset=UTF-8	No
2023-07-25 09:36:57	200	GET	http://wei.vialancer.com/	text/html; charset=UTF-8	No
2023-07-25 09:35:42	200	GET	http://wei.vialancer.com/	text/html; charset=UTF-8	No
2023-07-25 09:33:16	200	GET	http://wei.vialancer.com/	text/html; charset=UTF-8	No
2023-07-24 17:45:43	200	GET	http://wei.vialancer.com/	text/html; charset=UTF-8	No

View Data

Session User Data

Session doesn't seem to be active.

Request ( HTTP/1.1 )

$_GET

c	show
id	27

Headers

Cookie	pgv_pvi=2798497912
Accept-Language	zh-CN,zh;q=0.9
Accept-Encoding	gzip, deflate
Referer	http://wei.vialancer.com/index.php?c=category&id=12
Accept	text/html,application/xhtml+xml,application/xml;q=0.9,image/avif,image/webp,image/apng,/;q=0.8,application/signed-exchange;v=b3;q=0.7
User-Agent	Mozilla/5.0 (Windows NT 10.0; Win64; x64) AppleWebKit/537.36 (KHTML, like Gecko) Chrome/113.0.0.0 Safari/537.36
Upgrade-Insecure-Requests	1
Connection	keep-alive
Host	wei.vialancer.com

Cookies

pgv_pvi

2798497912

Response ( 200 - OK )

Headers

Cookie	pgv_pvi=2798497912
Accept-Language	zh-CN,zh;q=0.9
Accept-Encoding	gzip, deflate
Referer	http://wei.vialancer.com/index.php?c=category&id=12
Accept	text/html,application/xhtml+xml,application/xml;q=0.9,image/avif,image/webp,image/apng,/;q=0.8,application/signed-exchange;v=b3;q=0.7
User-Agent	Mozilla/5.0 (Windows NT 10.0; Win64; x64) AppleWebKit/537.36 (KHTML, like Gecko) Chrome/113.0.0.0 Safari/537.36
Upgrade-Insecure-Requests	1
Connection	keep-alive
Host	wei.vialancer.com

System Configuration

Read the CodeIgniter docs...

CodeIgniter Version:	4.0.5
PHP Version:	7.2.16
PHP SAPI:	fpm-fcgi
Environment:	development
Base URL:	http://wei.vialancer.com/
Timezone:	PRC
Locale:	en
Content Security Policy Enabled:	No